Abstract
A series of Al x Ga 1-x N/AlN/Sapphire films with x = 0.35–0.75 and different thickness of epi-layer were prepared by metalorganic chemical vapor deposition (MOCVD). Spectroscopic ellipsometry (SE) was used to study the temperature-dependent refractive indices and optical bandgaps of the Al x Ga 1-x N films ranging from 300 to 823 K. Parametric semiconductor (PSEMI) models were used to describe the dielectric functions of AlGaN/AlN layers. The fitting results of refractive index, energy bandgap, thickness and surface roughness at 300 K are in good agreement with photoluminescence (PL), scanning electron microscopy (SEM) measurements and the existing literature. Our finding indicates that the crystal quality of the samples with x = 0.47 and 0.60 are better than those with x = 0.35 and 0.75. As the temperature rises, the increasing of refractive index for the low Al content Al x Ga 1-x N layers is stronger than that of high Al content in the transparent region, and the reduction of bandgap with high Al content is larger than that of low Al content. For all the samples (x = 0.35–0.75), an analytical expression for temperature-dependent refractive index in the wavelength range of 195–1650 nm was obtained using the Sellmeier law, and the quantitative analysis of the SE-derived temperature-dependent bandgap was conducted by using the Bose-Einstein equation.
Recommended Citation
Y. Liu and Q. X. Li and L. Y. Wan and B. Kucukgok and E. Ghafari and I. T. Ferguson and X. Zhang and S. Wang and Z. C. Feng and N. Lu, "Composition and Temperature Dependent Optical Properties of Al x Ga 1-x N Alloy by Spectroscopic Ellipsometry," Applied Surface Science, vol. 421, pp. 389 - 396, Elsevier, Nov 2017.
The definitive version is available at https://doi.org/10.1016/j.apsusc.2017.01.309
Department(s)
Electrical and Computer Engineering
Keywords and Phrases
Al Ga N x 1-x; Optical properties; Spectroscopic ellipsometry; Temperature
International Standard Serial Number (ISSN)
0169-4332
Document Type
Article - Journal
Document Version
Citation
File Type
text
Language(s)
English
Rights
© 2024 Elsevier, All rights reserved.
Publication Date
01 Nov 2017
Comments
National Natural Science Foundation of China, Grant 2013GXNSFFA019001