Abstract

The rotational barrier about the CN carbamate bond of N-(4-hydroxybutyl)-N-(2,2,2-trifluoroethyl) tert-butyl carbamate 1 was determined by variable temperature (VT) 13C and 19F NMR spectroscopy. The −CH2CF3 appendage reports on rotational isomerism and allows for the observation of separate signals for the E- and Z-ensembles at low temperature. The activation barrier for E/Z-isomerization was quantified using Eyring-Polanyi theory which requires the measurements of the maximum difference in Larmor frequency Δνmax and the convergence temperature Tc. Both Δνmax and Tc were interpolated by analyzing sigmoidal functions fitted to data describing signal separation and the quality of the superposition of the E- and Z-signals, respectively. Methods for generating the quality-of-fit parameters for Lorentzian line shape analysis are discussed. Our best experimental value for the rotational barrier ΔGc≠(1)=15.65±0.13 kcal/mol is compared to results of a higher level ab initio study of the model N-ethyl-N-(2,2,2-trifluoroethyl) methyl carbamate.

Department(s)

Chemistry

Publication Status

Full Access

Comments

National Science Foundation, Grant 1665487

Keywords and Phrases

E/Z-Isomerization; Eyring-Polanyi Equation; Fluorinated Carbamates; Lorentzian Line Fitting; Variable Temperature NMR Spectroscopy

International Standard Serial Number (ISSN)

2365-6549

Document Type

Article - Journal

Document Version

Citation

File Type

text

Language(s)

English

Rights

© 2024 Wiley, All rights reserved.

Publication Date

24 Apr 2024

Included in

Chemistry Commons

Share

 
COinS