Abstract

The optical responses of monolayer transition metal dichalcogenides (1L-TMDs) can be tuned effectively by using mechanical strain. In this work, the tuning of upconversion photoluminescence (UPL) emission in 1L-WSSe alloy by applying uniaxial tensile strain is investigated. When the uniaxial tensile strain is changed from 0 % to 1.02 %, the peak position of UPL emission has a redshift of around 25.6 nm, and the UPL intensity goes up with an exponential function of the applied strain as the upconversion energy difference is varied from −197 meV to −131 meV. The sublinear power dependence for UPL emission in 1L-WSSe alloy indicates the multiphonon-mediated upconversion emission process involved with one photon. The demonstrated strain-tunable UPL emission in 1L-TMD alloys will advance potential applications in upconversion photonic devices and flexible optoelectronics.

Department(s)

Mechanical and Aerospace Engineering

Publication Status

Full Text Access

Comments

Defense Advanced Research Projects Agency, Grant W911NF2110353

Keywords and Phrases

Uniaxial tensile strain; Upconversion photoluminescence; WSSe alloy monolayer

International Standard Serial Number (ISSN)

0925-3467

Document Type

Article - Journal

Document Version

Citation

File Type

text

Language(s)

English

Rights

© 2026 Elsevier, All rights reserved.

Publication Date

01 Jan 2026

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