Influence Of Severe Plastic Deformation Processing On Grain Refinement And Neutron Irradiation Response In FeCrAl Alloys

Abstract

Grain boundary engineering enables radiation-tolerant structural materials by using refined grain size to absorb irradiation-induced defects. In this study, we explore this concept in FeCrAl alloys, promising candidates for accident-tolerant fuel cladding in light-water reactors due to their exceptional high-temperature oxidation resistance. However, a comprehensive understanding of their behavior under neutron irradiation, especially the effect of grain size on radiation tolerance, is still lacking. Here, the commercial FeCrAl alloy Kanthal D was subjected to severe plastic deformation via equal-channel angular pressing (ECAP) and high-pressure torsion (HPT) to produce ultrafine-grained (UFG, 100 nm–1 μm) and nanocrystalline (NC, <100 nm) microstructures, respectively. These processed materials, along with coarse-grained (CG) counterparts, were neutron irradiated to 2.6 to 3.2 displacements per atom (dpa) at approximately 358 °C and 554 °C. Post-irradiation mechanical testing revealed that the UFG and NC samples retained a more favorable combination of strength and ductility compared to the irradiated CG material, particularly after irradiation at 554 °C. The improved post-irradiation mechanical response of the UFG and NC conditions is attributed to the combined influence of SPD-induced grain refinement and associated microstructural features, rather than grain size alone. Increased grain-boundary density, deformation-induced dislocation structures, grain-boundary character, and recovery processes likely contribute to altered defect accumulation and reduced embrittlement relative to the CG condition. These findings highlight the potential of SPD-based microstructural engineering as a pathway for improving the neutron irradiation response of FeCrAl alloys.

Department(s)

Materials Science and Engineering

Comments

Idaho Operations Office, U.S. Department of Energy, Grant DE-NE0008524

International Standard Serial Number (ISSN)

0921-5093

Document Type

Article - Journal

Document Version

Citation

File Type

text

Language(s)

English

Rights

© 2026 Elsevier, All rights reserved.

Publication Date

01 Nov 2026

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