Abstract

Temperature and composition dependences of high-energy longitudinal optical (LO) phonons in YBa2Cu3O6+x, studied by inelastic neutron scattering measurements, provide clear evidence for temperature dependent spatial inhomogeneity of doped charges. The measurements indicate that charge doping increases the volume fraction of the charged regions, while the local charge density remains unchanged. For the optimally doped sample the charge distribution changes sharply near the superconducting transition temperature, with stronger charge inhomogeneity below TC. The remarkable magnitude of the phonon response to charge suggests strong involvement of phonons in charge dynamics.

Department(s)

Materials Science and Engineering

Comments

The authors are grateful to A. R. Bishop, V. J. Emery, L. P. Gor’kov, A. Bussmann-Holder, and V. Kresin for useful discussions. The research at University of Pennsylvania was supported by the National Science Foundation through DMR96-28136. Measurements were made at Oak Ridge National Laboratory, which is managed by Lockheed Martin Energy Research under contract no. DE-AC05-96OR22464 for the Department of Energy.

Document Type

Article - Journal

Document Version

Preprint

File Type

text

Language(s)

English

Publication Date

2018-10-28

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