Design of Ultra-High Temperature Ceramic Nano-Composites from Multi-Scale Length Microstructure Approach

Abstract

The evolution of the multi-scale microstructure of a (Zr,Ta)B2 solid solution was studied as a function of time and temperature. The ceramics were produced by hot pressing a mixture of ZrB2 with 15 vol% TaSi2 followed by annealing at 2100 °C. Formation of a super-saturated solid solution led to the precipitation of TaC nano-needles within the micron-sized boride grain matrix. Phase stability diagrams were used to define the conditions of partial pressure within the sintering chamber that drove precipitation of nano-inclusions in the form of either metal or carbide. Through this approach, other systems containing various transition metals were explored to design other formulations for in-situ nano-composites with unprecedented strength at ultra-elevated temperatures.

Department(s)

Materials Science and Engineering

Comments

This research was partially sponsored by the NATO Science for Peace and Security Programme under grant MYP-G5767 (SUSPENCE) and by the US AFOSR through the Cooperative Agreement no. FA9550-21-1-0399 (NACREOUS) with Dr. Ming-Jen Pan as contract monitor.

Keywords and Phrases

Core-Shell; Electron Microscopy; Interface/Interphase; Nano-Structures; Sintering

International Standard Serial Number (ISSN)

1359-8368

Document Type

Article - Journal

Document Version

Citation

File Type

text

Language(s)

English

Rights

© 2021 Elsevier, All rights reserved.

Publication Date

01 Dec 2021

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