Characterization of Alloy Particles Extracted from Spent Nuclear Fuel

Abstract

We characterized, for the first time, submicro- and nanosized fission product-alloy particles that were extracted nondestructively from spent nuclear fuel, in terms of noble metal (Mo-Ru-Tc-Rh-Pd-Te) composition, atomic level homogeneity and lattice parameters. The evidences obtained in this work contribute to an improved understanding of the redox chemistry of radionuclides in nuclear waste repository environments and, in particular, of the catalytic properties of these unique metal alloy particles.

Department(s)

Geosciences and Geological and Petroleum Engineering

Keywords and Phrases

Alloy Particles; Atomic Levels; Catalytic Properties; Metal Alloys; Nano-Sized; Nuclear Waste Repositories; Redox Chemistry; Spent Nuclear Fuels; Alloys; Fission Products; Geological Repositories; Palladium; Precious Metals; Radioactive Wastes; Rhodium; Ruthenium Alloys; Molybdenum

International Standard Serial Number (ISSN)

0022-3115

Document Type

Article - Journal

Document Version

Citation

File Type

text

Language(s)

English

Rights

© 2012 Elsevier, All rights reserved.

Publication Date

01 Jan 2012

Share

 
COinS