Abstract

The electrophoretic transport of three chemically reacting species, two of which can bind reversibly to form the third, is analyzed mathematically. The species are assumed to move horizontally through a long channel with different electrophoretic mobilities and diffusion coefficients. By considering small perturbations of the system about equilibrium or when one of the two binding species is much more abundant than the other, the governing advection-reaction- diffusion equations can be linearized and studied via the method of moments. The result is a set of coupled ordinary differential equations for the moments that can be solved analytically. Analysis of the long-time evolution of the moments yields mean velocities and dispersion coefficients for each species. The results provide a method for measuring the rate and equilibrium constants of binding reactions using capillary electrophoresis. © 2007 The American Physical Society.

Department(s)

Business and Information Technology

Second Department

Chemical and Biochemical Engineering

International Standard Serial Number (ISSN)

1550-2376; 1539-3755

Document Type

Article - Journal

Document Version

Citation

File Type

text

Language(s)

English

Rights

© 2025 American Physical Society, All rights reserved.

Publication Date

30 Nov 2007

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