Recent measurements have examined the electron-impact ionization of excited-state laser-aligned Mg atoms. In this work we show that the ionization cross section arising from the geometry where the aligned atom is perpendicular to the scattering plane directly probes the unnatural parity contributions to the ionization amplitude. The contributions from natural parity partial waves cancel exactly in this geometry. Our calculations resolve the discrepancy between the nonzero measured cross sections in this plane and the zero cross section predicted by distorted-wave approaches. We demonstrate that this is a general feature of ionization from p-state targets by additional studies of ionization from excited Ca and Na atoms.
G. S. Armstrong et al., "Evidence for Unnatural-Parity Contributions to Electron-Impact Ionization of Laser-Aligned Atoms," Physical Review A - Atomic, Molecular, and Optical Physics, vol. 92, no. 3, American Physical Society (APS), Sep 2015.
The definitive version is available at https://doi.org/10.1103/PhysRevA.92.032706
Center for High Performance Computing Research
Keywords and Phrases
Atom Lasers; Atoms; Electron Scattering; Excited States; Ionization; Ionization of Gases; Distorted Waves; Electron Impact-Ionization; Ionization Amplitude; Ionization Cross Section; Na Atoms; Partial Waves; Scattering Plane; Impact Ionization
International Standard Serial Number (ISSN)
Article - Journal
© 2015 American Physical Society (APS), All rights reserved.
01 Sep 2015