Doctoral Dissertations

Author

Jie Li

Keywords and Phrases

Additive Manufacturing; Battery Management System; Li-Ion Battery

Abstract

"The applications of Li-ion batteries require higher energy and power densities, improved safety, and sophisticated battery management systems. To satisfy these demands, as battery performances depend on the network of constituent materials, it is necessary to optimize the electrode structure. Simultaneously, the states of the battery have to be accurately estimated and controlled to maintain a durable condition of the battery system. For those purposes, this research focused on the innovation of 3D electrode via additive manufacturing, and the development of fast and accurate physical based models to predict the battery status for control purposes. Paper I proposed a novel 3D structure electrode, which exhibits both high areal and specific capacity, overcoming the trade-off between the two of the conventional batteries. Paper II proposed a macro-micro-controlled Li-ion 3D battery electrode. The battery structure is controlled by electric fields at the particle level to increase the aspect ratio and then improve battery performance. Paper III introduced a 3D model to simulate the electrode structure. The effect of electrode thickness and solid phase volume fraction were systematically studied. Paper IV proposed a low-order battery model that incorporates stress-enhanced diffusion and electrolyte physic into a Single Particle model that addresses the challenges of battery modeling for BMS: accuracy and computational efficiency. Paper V proposed a single particle-based degradation model by including Solid Electrolyte Interface (SEI) layer formation coupled with crack propagation. Paper VI introduced a single-particle-based degradation model by considering the dissolution of active materials and the Li-ion loss due to SEI layer formation with crack propagation for LiMn₂O₄/Graphite battery"--Abstract, page iv.

Advisor(s)

Park, Jonghyun

Committee Member(s)

Landers, Robert G.
Leu, M. C. (Ming-Chuan)
Wojnar, Charles
Liang, Xinhua

Department(s)

Mechanical and Aerospace Engineering

Degree Name

Ph. D. in Mechanical Engineering

Publisher

Missouri University of Science and Technology

Publication Date

Summer 2018

Journal article titles appearing in thesis/dissertation

  • A hybrid three-dimensionally structured electrode for lithium-ion batteries via 3D printing
  • Macro-/micro-controlled lithium-ion 3D battery via 3D printing and electric field
  • Enhanced battery performance through 3D structured electrodes: Experimental and modeling study
  • A single particle model for lithium-ion batteries with electrolyte and stress-enhanced diffusion physics
  • A single particle model with chemical/mechanical degradation physics for lithium ion battery state of health (SOH) estimation
  • A single particle-based battery degradation model and life estimation for LiMn₂O₄/graphite battery

Pagination

xvii, 191 pages

Note about bibliography

Includes bibliographic references.

Rights

© 2018 Jie Li, All rights reserved.

Document Type

Dissertation - Open Access

File Type

text

Language

English

Thesis Number

T 11384

Electronic OCLC #

1051223117

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