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Title: Enhancing Enantioselectivity of Electrodeposited CuO Films by Chiral Etching
Department/Lab Affiliations: Chemistry
Materials Research Center
Materials Science & Engineering
Keywords: Chiral Etching
Cyclic voltammetry
Electrodeposited
Enantioselectivity
Issue Date: 2007
Publisher: American Chemical Society ACS
Citation: Shaibal K. Sarkar, Niharika Burla, Eric W. Bohannan, and Jay A. Switzer. Enhancing Enantioselectivity of Electrodeposited CuO Films by Chiral Etching, Journal of the American Chemical Society, Vol. 129(29), pp. 8972-8973, 2007
Abstract: The enantioselectivity of electrodeposited CuO with a chiral orientation is enhanced if the CuO is first etched in a solution of tartaric acid. Electrochemical quartz crystal microbalance studies show that CuO(1) electrodeposited from L-tartrate etches faster in L-tartaric acid, whereas CuO(1) electrodeposited from D-tartrate etches faster in D-tartaric acid. The enantioselectivity is probed by cyclic voltammetry. The proposed mechanism differentiates between chiral orientation and chiral surface. The enhancement of enantioselectivity of the films with chiral orientations is attributed to an increase in the chiral surface area of the etched CuO films.
Type: Article
text
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titleEnhancing Enantioselectivity of Electrodeposited CuO Films by Chiral Etching
contributorBohannan, Eric
contributorSwitzer, Jay A.
contributorSarkar, Shaibal K.
contributorBurla, Niharika
contributor.deptlabChemistry
contributor.deptlabMaterials Research Center
contributor.deptlabMaterials Science & Engineering
contributor.sponsorNational Science Foundation
subjectChiral Etching
subjectCyclic voltammetry
subjectElectrodeposited
subjectEnantioselectivity
date.issued2007
publisherAmerican Chemical Society ACS
identifier.citationShaibal K. Sarkar, Niharika Burla, Eric W. Bohannan, and Jay A. Switzer. Enhancing Enantioselectivity of Electrodeposited CuO Films by Chiral Etching, Journal of the American Chemical Society, Vol. 129(29), pp. 8972-8973, 2007
identifier.pubhttp://dx.doi.org/10.1021/ja073640b
description.abstractThe enantioselectivity of electrodeposited CuO with a chiral orientation is enhanced if the CuO is first etched in a solution of tartaric acid. Electrochemical quartz crystal microbalance studies show that CuO(1) electrodeposited from L-tartrate etches faster in L-tartaric acid, whereas CuO(1) electrodeposited from D-tartrate etches faster in D-tartaric acid. The enantioselectivity is probed by cyclic voltammetry. The proposed mechanism differentiates between chiral orientation and chiral surface. The enhancement of enantioselectivity of the films with chiral orientations is attributed to an increase in the chiral surface area of the etched CuO films.
typeArticle
type.DCMITypetext
rightsPre-print: author cannot archive; Post-print: author cannot archive;
rightsThis material is presented to ensure timely dissemination of scholarly and technical work. Copyright and all rights therein are retained by authors or by other copyright holders. All persons copying this information are expected to adhere to the terms and constraints invoked by each author's copyright. In most cases, these works may not be reposted without the explicit permission of the copyright holder.
rights.URI
http://pubs.acs.org/copyright/nih/
rights.URI
http://pubs.acs.org/instruct/copyright.pdf
date.available2008-07-01T21:33:58Z
identifier.persist.URI
http://scholarsmine.mst.edu/post_prints/EnhancingEnantioselectivityOfElectrodepositedC_09007dcc80526abd.html