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Title: Electrochemical biomineralization: the deposition of calcite with chiral morphologies
Author (s): Kulp, Elizabeth
Switzer, Jay A.
Department/Lab Affiliations: Chemistry
Materials Research Center
Materials Science & Engineering
Keywords: aragonite
calcite
chiral morphologies
Issue Date: 2007
Publisher: American Chemical Society ACS
Citation: Elizabeth A. Kulp and Jay A. Switzer. Electrochemical Biomineralization: the Deposition of Calcite with Chiral Morphologies, Journal of the American Chemical Society, Vol. 129(49), pp. 15120-15121, 2007
Abstract: The biominerals calcite and aragonite are electrodeposited by electrochemically generating base in a solution containing Ca2+ and HCO3-. Although calcite crystallizes in the achiral space group Rc, orientations of calcite which lack mirror or glide plane symmetry are chiral. Chiral morphologies of calcite are electrodeposited in the presence of tartaric, malic, and aspartic acid. Calcite grows with left-handed spirals when deposited from L-tartaric acid but grows with right-handed spirals when deposited from L-malic acid or L-aspartic acid. A racemic mixture of D- and L-malic acid produces an achiral microstructure, instead of producing a racemic mixture of chiral microstructures.
Type: Article
text
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http://pubs.acs.org/copyright/nih/
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Publisher URL:
http://dx.doi.org/10.1021/ja076303b
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titleElectrochemical biomineralization: the deposition of calcite with chiral morphologies
contributor.authorKulp, Elizabeth
contributor.authorSwitzer, Jay A.
contributor.deptlabChemistry
contributor.deptlabMaterials Research Center
contributor.deptlabMaterials Science & Engineering
contributor.sponsorNational Science Foundation
subjectaragonite
subjectcalcite
subjectchiral morphologies
date.issued2007
publisherAmerican Chemical Society ACS
identifier.citationElizabeth A. Kulp and Jay A. Switzer. Electrochemical Biomineralization: the Deposition of Calcite with Chiral Morphologies, Journal of the American Chemical Society, Vol. 129(49), pp. 15120-15121, 2007
identifier.pub.URI
http://dx.doi.org/10.1021/ja076303b
description.abstractThe biominerals calcite and aragonite are electrodeposited by electrochemically generating base in a solution containing Ca2+ and HCO3-. Although calcite crystallizes in the achiral space group Rc, orientations of calcite which lack mirror or glide plane symmetry are chiral. Chiral morphologies of calcite are electrodeposited in the presence of tartaric, malic, and aspartic acid. Calcite grows with left-handed spirals when deposited from L-tartaric acid but grows with right-handed spirals when deposited from L-malic acid or L-aspartic acid. A racemic mixture of D- and L-malic acid produces an achiral microstructure, instead of producing a racemic mixture of chiral microstructures.
typeArticle
type.DCMITypetext
rightsPre-print: author cannot archive; Post-print: author cannot archive;
rightsThis material is presented to ensure timely dissemination of scholarly and technical work. Copyright and all rights therein are retained by authors or by other copyright holders. All persons copying this information are expected to adhere to the terms and constraints invoked by each author's copyright. In most cases, these works may not be reposted without the explicit permission of the copyright holder.
rights.URI
http://pubs.acs.org/copyright/nih/
rights.URI
http://pubs.acs.org/instruct/copyright.pdf
date.available2008-07-01T21:24:19Z
identifier.persist.URI
http://scholarsmine.mst.edu/post_prints/ElectrochemicalBiomineralizationTheDepositionOf_09007dcc80526a27.html