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Title: Oxidase-coupled amperometric glucose and lactate sensors with integrated electrochemical actuation system
Author (s): Jongwon Park
Kim, Chang-Soo
Choi, Minsu
Department/Lab Affiliations: Biological Sciences
Electrical and Computer Engineering
Intelligent Microsystem Laboratory
Keywords: Actuator
amperometric sensors
baseline drift
biosensors
calibration
electrochemical actuation system
electrolytic generation
enzyme activity
enzymes
glucose oxidase
glucose oxidase (GOD)
lactate oxidase
lactate oxidase (LOD)
oxidase enzyme
sensitivity
sensitivity degradation
sensors diagnosis
solid-state biosensor
sugar
thin-film amperometric sensor
water electrolysis
Issue Date: 2006
Publisher: Institute of Electrical and Electronics Engineers
Citation: Jongwon Park; Chang-Soo Kim; Minsu Choi, "Oxidase-coupled amperometric glucose and lactate sensors with integrated electrochemical actuation system" IEEE Transactions on Instrumentation and Measurement, vol.55, no.4 pp. 1348- 1355, Aug. 2006
Abstract: Unpredictable baseline drift and sensitivity degradation during continuous use are two of the most significant problems of biosensors including the amperometric glucose and lactate sensors. Therefore, the capability of on-demand in situ calibration/diagnosis of biochemical sensors is indispensable for reliable long-term monitoring with minimum attendance. Another limitation of oxidase enzyme-based biosensors is the dependence of enzyme activity on the background oxygen concentration in sample solution. In order to address these issues, the electrolytic generation of oxygen and hydrogen bubbles were utilized 1) to overcome the background oxygen dependence of glucose and lactate sensors and 2) to demonstrate the feasibility of in situ self-calibration of the proposed glucose and lactate sensors. Experimental data assure that the proposed techniques effectively establish the zero calibration value and significantly improve the measurement sensitivity and dynamic range in both glucose and lactate sensors.
Type: Article - Journal
text
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titleOxidase-coupled amperometric glucose and lactate sensors with integrated electrochemical actuation system
contributor.authorJongwon Park
contributor.authorKim, Chang-Soo
contributor.authorChoi, Minsu
contributor.deptlabBiological Sciences
contributor.deptlabElectrical and Computer Engineering
contributor.deptlabIntelligent Microsystem Laboratory
subjectActuator
subjectamperometric sensors
subjectbaseline drift
subjectbiosensors
subjectcalibration
subjectelectrochemical actuation system
subjectelectrolytic generation
subjectenzyme activity
subjectenzymes
subjectglucose oxidase
subjectglucose oxidase (GOD)
subjectlactate oxidase
subjectlactate oxidase (LOD)
subjectoxidase enzyme
subjectsensitivity
subjectsensitivity degradation
subjectsensors diagnosis
subjectsolid-state biosensor
subjectsugar
subjectthin-film amperometric sensor
subjectwater electrolysis
date.issued2006
date.submitted2007
publisherInstitute of Electrical and Electronics Engineers
identifier.citationJongwon Park; Chang-Soo Kim; Minsu Choi, "Oxidase-coupled amperometric glucose and lactate sensors with integrated electrochemical actuation system" IEEE Transactions on Instrumentation and Measurement, vol.55, no.4 pp. 1348- 1355, Aug. 2006
identifier.issn0018-9456
identifier.pub.URI
http://ieeexplore.ieee.org/iel5/19/34720/01658390.pdf?arnumber=165839
description.abstractUnpredictable baseline drift and sensitivity degradation during continuous use are two of the most significant problems of biosensors including the amperometric glucose and lactate sensors. Therefore, the capability of on-demand in situ calibration/diagnosis of biochemical sensors is indispensable for reliable long-term monitoring with minimum attendance. Another limitation of oxidase enzyme-based biosensors is the dependence of enzyme activity on the background oxygen concentration in sample solution. In order to address these issues, the electrolytic generation of oxygen and hydrogen bubbles were utilized 1) to overcome the background oxygen dependence of glucose and lactate sensors and 2) to demonstrate the feasibility of in situ self-calibration of the proposed glucose and lactate sensors. Experimental data assure that the proposed techniques effectively establish the zero calibration value and significantly improve the measurement sensitivity and dynamic range in both glucose and lactate sensors.
typeArticle - Journal
type.DCMITypetext
type.statusFinal version
rightsThis material is presented to ensure timely dissemination of scholarly and technical work. Copyright and all rights therein are retained by authors or by other copyright holders. All persons copying this information are expected to adhere to the terms and constraints invoked by each author's copyright. In most cases, these works may not be reposted without the explicit permission of the copyright holder.
rights.URI
http://www.ieee.org/web/publications/rights/policies.html
date.accessioned2007-04-05T14:27:22Z
date.available2007-04-05T14:27:22Z
identifier.persist.URI
http://scholarsmine.mst.edu/post_prints/01658390_09007dcc8030da8f.html
Full Text
01658390_09007dcc8030da94.pdf