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Title: Study of structural and magnetic properties of iron-rich mixed rare-Earth NdDyFe (17-y-x)CoxSiy compounds
Author (s): Kamaraju, K.
Yang, J.B.
Yelon, William B.
Pringle, O. Allan
Kim, M.
James, William Joseph
Cai, Q.
Department/Lab Affiliations: Chemistry
Physics
Keywords: 305 to 405 degC
Curie temperature
Curie temperatures
DH
DR
Disordered hexagonal
NdDyFe(17-y-x)CoxSiy
Rietveld program
cobalt alloys
disordered hexagonal structure
disordered rhombohedral structure
disordered rhomboherdral
dysprosium alloys
ferromagnetic materials
high-purity elements
induction melting
iron
iron alloys
magnetic annealing
magnetic ordering transition temperature
magnetic properties
magnetization
neodymium alloys
permanent magnets
rare-Earth materials
silicon alloys
solid solutions
structural study
Issue Date: 2004
Publisher: Institute of Electrical and Electronics Engineers
Citation: Kamaraju, K.; Yang, J.B.; Yelon, W.B.; Pringle, O.A.; Kim, M.; James, W.J.; Cai, Q. "Study of structural and magnetic properties of iron-rich mixed rare-Earth NdDyFe(17-y-x)CoxSiy compounds" IEEE Transactions on Magnetics, Vol.40, Iss.4, July 2004 Pages: 2910- 2912
Abstract: A series of NdDyFe(17-y-x)CoxSiy solid solutions with = 2 and 3 and = 0.5 1.0 and 1.5 were prepared by induction melting stoichiometric amounts of high-purity elements. The postannealed samples consist of two phases belonging to the space groups R3 m and P63 mmc . The lattice parameters and the unit cell volumes were calculated from the refinements of the magnetic and structural unit cells using the FULLPROF version of the Rietveld program. For a fixed content of Co, the maximum Curie temperatures (305 C to 405 C) were observed in samples with = 1 and having two phases, a disordered rhombohedral (DR) structure and a disordered hexagonal (DH) structure. An increase in the Curie temperature of 70 C per atom of cobalt is observed in NdDyFe(17-y-x)CoxSiy with y = 1 and x< 3, suggesting that with a suitable choice of rare earths this DR phase may be a promising candidate for high-energy product permanent magnets. The magnetization versus temperature (M versus T) plots of the solid solutions, which consist of two phases, exhibit only a single magnetic ordering transition temperature.
Type: Article - Journal
text
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titleStudy of structural and magnetic properties of iron-rich mixed rare-Earth NdDyFe (17-y-x)CoxSiy compounds
contributor.authorKamaraju, K.
contributor.authorYang, J.B.
contributor.authorYelon, William B.
contributor.authorPringle, O. Allan
contributor.authorKim, M.
contributor.authorJames, William Joseph
contributor.authorCai, Q.
contributor.deptlabChemistry
contributor.deptlabElectronic Materials Applied Research Center
contributor.deptlabPhysics
subject305 to 405 degC
subjectCurie temperature
subjectCurie temperatures
subjectDH
subjectDR
subjectDisordered hexagonal
subjectNdDyFe(17-y-x)CoxSiy
subjectRietveld program
subjectcobalt alloys
subjectdisordered hexagonal structure
subjectdisordered rhombohedral structure
subjectdisordered rhomboherdral
subjectdysprosium alloys
subjectferromagnetic materials
subjecthigh-purity elements
subjectinduction melting
subjectiron
subjectiron alloys
subjectmagnetic annealing
subjectmagnetic ordering transition temperature
subjectmagnetic properties
subjectmagnetization
subjectneodymium alloys
subjectpermanent magnets
subjectrare-Earth materials
subjectsilicon alloys
subjectsolid solutions
subjectstructural study
date.issued2004
date.submitted2007
publisherInstitute of Electrical and Electronics Engineers
identifier.citationKamaraju, K.; Yang, J.B.; Yelon, W.B.; Pringle, O.A.; Kim, M.; James, W.J.; Cai, Q. "Study of structural and magnetic properties of iron-rich mixed rare-Earth NdDyFe(17-y-x)CoxSiy compounds" IEEE Transactions on Magnetics, Vol.40, Iss.4, July 2004 Pages: 2910- 2912
identifier.issn0018-9464
identifier.pub.URI
http://ieeexplore.ieee.org/iel5/20/29331/01325682.pdf?arnumber=132568
description.abstractA series of NdDyFe(17-y-x)CoxSiy solid solutions with = 2 and 3 and = 0.5 1.0 and 1.5 were prepared by induction melting stoichiometric amounts of high-purity elements. The postannealed samples consist of two phases belonging to the space groups R3 m and P63 mmc . The lattice parameters and the unit cell volumes were calculated from the refinements of the magnetic and structural unit cells using the FULLPROF version of the Rietveld program. For a fixed content of Co, the maximum Curie temperatures (305 C to 405 C) were observed in samples with = 1 and having two phases, a disordered rhombohedral (DR) structure and a disordered hexagonal (DH) structure. An increase in the Curie temperature of 70 C per atom of cobalt is observed in NdDyFe(17-y-x)CoxSiy with y = 1 and x< 3, suggesting that with a suitable choice of rare earths this DR phase may be a promising candidate for high-energy product permanent magnets. The magnetization versus temperature (M versus T) plots of the solid solutions, which consist of two phases, exhibit only a single magnetic ordering transition temperature.
typeArticle - Journal
type.DCMITypetext
type.statusFinal version
rightsThis material is presented to ensure timely dissemination of scholarly and technical work. Copyright and all rights therein are retained by authors or by other copyright holders. All persons copying this information are expected to adhere to the terms and constraints invoked by each author's copyright. In most cases, these works may not be reposted without the explicit permission of the copyright holder.
rights.URI
http://www.ieee.org/web/publications/rights/policies.html
date.accessioned2007-04-05T14:20:20Z
date.available2007-04-05T14:20:20Z
identifier.persist.URI
http://scholarsmine.mst.edu/post_prints/01325682_09007dcc8030d26c.html
Full Text
01325682_09007dcc8030d271.pdf