Anomalous Length Dependence of the Quantum Yield in Artificial Photosynthetic Systems

Abstract

We show that the quantum yield in an artificial N-site photosynthetic system can be calculated exactly if e--hole recombination is allowed from the light absorber only. It is then demonstrated that the distribution of hopping rates determined the N dependence of the quantum yield and may give rise to a faster than 1/N decay of the quantum yield.

Department(s)

Physics

International Standard Serial Number (ISSN)

0009-2614

Document Type

Article - Journal

Document Version

Citation

File Type

text

Language(s)

English

Rights

© 1988 Elsevier, All rights reserved.

Publication Date

01 Sep 1988

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