Anomalous Length Dependence of the Quantum Yield in Artificial Photosynthetic Systems
We show that the quantum yield in an artificial N-site photosynthetic system can be calculated exactly if e--hole recombination is allowed from the light absorber only. It is then demonstrated that the distribution of hopping rates determined the N dependence of the quantum yield and may give rise to a faster than 1/N decay of the quantum yield.
K. P. Kundu et al., "Anomalous Length Dependence of the Quantum Yield in Artificial Photosynthetic Systems," Chemical Physics Letters, vol. 150, no. 1-2, pp. 174-176, Elsevier, Sep 1988.
The definitive version is available at http://dx.doi.org/10.1016/0009-2614(88)80417-2
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