First-Principles Electron Dynamics Control Simulation of Diamond under Femtosecond Laser Pulse Train Irradiation

Abstract

A real-time and real-space time-dependent density functional is applied to simulate the nonlinear electronphoton interactions during shaped femtosecond laser pulse train ablation of diamond. Effects of the key pulse train parameters such as the pulse separation, spatial/temporal pulse energy distribution and pulse number per train on the electron excitation and energy absorption are discussed. The calculations show that photonelectron interactions and transient localized electron dynamics can be controlled including photon absorption, electron excitation, electron density, and free electron distribution by the ultrafast laser pulse train. © 2012 IOP Publishing Ltd.

Department(s)

Mechanical and Aerospace Engineering

Second Department

Electrical and Computer Engineering

Document Type

Article - Journal

Document Version

Citation

File Type

text

Language(s)

English

Rights

© 2012 Institute of Physics - IOP Publishing, All rights reserved.

Publication Date

01 Jan 2012

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